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Apart from cleaning up the /boot partition by removing kernels, you can still resize the LVM partitions by booting up a Live CD. You can use anything you want to resize the partition, with GUIs like gparted or CLI tools using lvresize.

This should be a useful guide: https://unix.stackexchange.com/questions/293148/how-to-reduce-lvm-for-root-partition. It'll work for /boot as well.